Really depends on the genre you're into..
Series I've enjoyed that I haven't seen mentioned:
Action type:
Code Geass + R2
Full Metal Alchemist (Brotherhood)
Claymore
Fate/Stay Night
Comedy/Drama:
Kanon
Clannad + AfterStory
Angel Beats
Also I would suggest holding off on...
Mount & Blade Warband is amazingly fun and addictive, also a fairly active mod community. Not a lot of story though if that's what you're looking for...
Mass Effect, Dragon Age etc. if you want a RPG with story.
Fallout 3, Obvlion etc are also good open ended RPGs
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