While I'm tempted to say Cowboy Bebop (Ba-dup Ba-dup Ba-dup Ba-dup BA-DOW!), I will have to go with Tengen Toppa Gurren Lagann. I watched the entire series via terrible Youtube quality (too poor to afford purchasing it and I don't even know where it's sold ;_
and my jaw was still hanging open in shock AT LEAST once per episode, and by the final I was locked in a permanent "OH SHI-" expression. Just amazing.
And yes, I realise both of these have been mentioned plenty of times already, but their quality truly cannot be overstated.
And yes, I realise both of these have been mentioned plenty of times already, but their quality truly cannot be overstated.